@article{fdi:010080020, title = {{S}ources of particulate-matter air pollution and its oxidative potential in {E}urope}, author = {{D}aellenbach, {K}. {R}. and {U}zu, {G}a{\¨e}lle and {J}iang, {J}. {H}. and {C}assagnes, {L}. {E}. and {L}eni, {Z}. and {V}lachou, {A}. and {S}tefenelli, {G}. and {C}anonaco, {F}. and {W}eber, {S}. and {S}egers, {A}. and {K}uenen, {J}. {J}. {P}. and {S}chaap, {M}. and {F}avez, {O}. and {A}lbinet, {A}. and {A}ksoyoglu, {S}. and {D}ommen, {J}. and {B}altensperger, {U}. and {G}eiser, {M}. and {E}l {H}addad, {I}. and {J}affrezo, {J}. {L}. and {P}revot, {A}. {S}. {H}.}, editor = {}, language = {{ENG}}, abstract = {{P}articulate matter is a component of ambient air pollution that has been linked to millions of annual premature deaths globally(1-3). {A}ssessments of the chronic and acute effects of particulate matter on human health tend to be based on mass concentration, with particle size and composition also thought to play a part(4). {O}xidative potential has been suggested to be one of the many possible drivers of the acute health effects of particulate matter, but the link remains uncertain(5-8). {S}tudies investigating the particulate-matter components that manifest an oxidative activity have yielded conflicting results(7). {I}n consequence, there is still much to be learned about the sources of particulate matter that may control the oxidative potential concentration(7). {H}ere we use field observations and air-quality modelling to quantify the major primary and secondary sources of particulate matter and of oxidative potential in {E}urope. {W}e find that secondary inorganic components, crustal material and secondary biogenic organic aerosols control the mass concentration of particulate matter. {B}y contrast, oxidative potential concentration is associated mostly with anthropogenic sources, in particular with fine-mode secondary organic aerosols largely from residential biomass burning and coarse-mode metals from vehicular non-exhaust emissions. {O}ur results suggest that mitigation strategies aimed at reducing the mass concentrations of particulate matter alone may not reduce the oxidative potential concentration. {I}f the oxidative potential can be linked to major health impacts, it may be more effective to control specific sources of particulate matter rather than overall particulate mass. {O}bservations and air-quality modelling reveal that the sources of particulate matter and oxidative potential in {E}urope are different, implying that reducing mass concentrations of particulate matter alone may not reduce oxidative potential.}, keywords = {{EUROPE}}, booktitle = {}, journal = {{N}ature}, volume = {587}, numero = {7834}, pages = {414--419 + 14 p.}, ISSN = {0028-0836}, year = {2020}, URL = {https://www.documentation.ird.fr/hor/fdi:010080020}, }